Is there any way to increase the capacity of these?
Are there any upgrades available for the 3rd Gen iPod shuffle to go to 8GB or more?
Is this a good question?
no, there is no upgrade possibility.
as you dan see in the shuffle teardown/step 13:
The primary (and only) chip, which is a multi-layered stack containing the CPU, RAM, and 4GB of flash memory.
so there is no "simple" flash memory in the shuffle and that fact makes an upgrade impossible
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